Note: If the Taskbar path does not exist, skip this step and go to the next solution. 
If you’re using a company computer, go to C:\Users\Public\CompanyName\TaskBar.Navigate to C:\Users\UserName\AppData\Roaming\Microsoft\Internet Explorer\Quick Launch\User Pinned\TaskBar.Edit your taskbar settings directly from your user profile directory and check the results.
The OS may also associate certain apps with your user account. Keep in mind that major Windows 10 updates may override these settings, and you may need to repeat the same steps again.
Save the file, unpin the app again and restart your computer. For instance, if it’s Edge, remove the line adding Edge. Simply remove the line of the problematic app. Alternatively, you can also go to %userprofile%\AppData\Local\Microsoft\Windows\Shell and open the LayoutModification.xml file with Notepad. For example, other users solved the problem by removing the CustomTaskbarLayoutCollection PinListPlacement=”Replace” line. Remove all the customs lines and check the results. Type custom in the search box and press Enter. If the issue persists, use CTRL + F and search for all “custom” lines. Save the settings, close the file and then unpin the apps manually. To do this, you need to type line, and then type –> after that line. Navigate to C:\Users\Default\AppData\Local\Microsoft\Windows\Shell\LayoutModification.xml. Many users confirmed they solved this problem by editing the Layout XML file. Contact your IT admin for more information. That could explain why you can’t permanently unpin your apps. If you’re using a computer managed by an organization, maybe the domain policies prevent you from unpinning certain apps from the taskbar. Unpinned Apps Keep Coming Back to the Taskbar Check Domain Rules
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